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Development and application of innovative technologies for drinking water quality assurance in China

QU Jiuhui, YIN Chengqing, YANG Min, LIU Huijuan

《环境科学与工程前沿（英文）》 2007年 第1卷 第3期   页码 257-269 doi: 10.1007/s11783-007-0044-y

摘要： The continuously deteriorating quality of source water is threatening the safety of drinking water in China. Various efforts have been made to update water treatment processes to decrease the pollution problems of drinking water, such as protection of drinking water sources, enhancement of conventional treatment processes, and development of new or advanced treatment technologies. This paper reviews a variety of protection and remediation methods for drinking water sources, development and application of drinking water treatment technologies, new technologies for special pollutants removal from groundwater, and the latest research progress on water distribution systems in China. treatment plant improvement is the key to ensure the quality of drinking water. There have been many researches on innovative treatment technologies in China and they have been applied in quite a number of water treatment plants. These innovations include key technique development and combination of technologies in the scope of economic optimization. On the basis of water quality from the plant, the distribution system is also important. This paper describes the latest development in the above respects.

关键词： advanced treatment     economic optimization     Various     enhancement     improvement    

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Effects of water quality on the coagulation performances of humic acids irradiated with UV light

Wendong WANG,Qinghai FAN,Zixia QIAO,Qin YANG,Yabo WANG,Xiaochang WANG

《环境科学与工程前沿（英文）》 2015年 第9卷 第1期   页码 147-154 doi: 10.1007/s11783-014-0749-7

摘要： The presence of humic acid in drinking water treatment has received significant attention in recent years because of its adverse effects on the removal of many pollutants in coagulation. In this paper, the effects of water quality including pH, turbidity, alkalinity, and hardness on the removal of humic acid were investigated in a UV light hybridized coagulation process. Our results suggested that UV light radiation could effectively improve the removal rate of humic acid in coagulation under both neutral and basic conditions, and the variations of the selected water quality parameters had little adverse effect on the function of UV light. After UV light radiation, the removal rate of the nitro-humic acid (NHA) increased from 20% to 60% in coagulation, and increased further to 75% and 85% for the raw waters with 10.0 NTU kaolin and 100 mg·L hardness, respectively. In addition to NHA, the removal rates of the humic acid extracted from peat coal (PHA) and the humic acid provided by Japan metals and chemicals company (JHA) in coagulation were also improved, both in the range of 80%–90% after undergoing UV light radiation. By changing the radiation location from prior to coagulation to the flocculation process, similar experimental results were obtained. The formation of positive charged sites after UV light radiation was considered to be the primary factor that led to an enhanced removal of the humic acid in coagulation.

关键词： coagulation     drinking water     humic acid     UV light radiation     water quality    

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Occurrence of odor problems in drinking water of major cities across China

SUN Daolin,YU Jianwei,YANG Min,AN Wei,ZHAO Yunyun,LU Ning,YUAN Shengguang,ZHANG Dongqing

《环境科学与工程前沿（英文）》 2014年 第8卷 第3期   页码 411-416 doi: 10.1007/s11783-013-0577-1

摘要： A comprehensive investigation into the occurrence of odor problem at 111 drinking water treatment plants (DWTPs) in major cities across China was undertaken using both flavor profile analysis (FPA) and gas chromatography–mass spectrometry (GC-MS). Eighty percent of source water samples exhibited odor problems, characterized by earthy/musty (41%) and swampy/septic (36%) odors, while the occurrence rate was lower (45%) in the finished water. Source water from rivers exhibited more pollution-origin odors, such as the swampy/septic odor, while that from lakes and reservoirs exhibited more algae-origin odors, such as earthy/musty odors. The occurrence rate of 2-methylisoborneol (2-MIB) in the surface source water samples was 75%, with 7% of samples containing 2-MIB concentrations of over 10 ng·L . The earthy/musty odor in the lake/reservoir water samples was mainly caused by 2-MIB (linear regression coefficient, =0.69), while the correlation between 2-MIB concentration and the earthy/musty odor intensity in the river-source water samples was weak ( =0.35). These results will be useful for the management of odor-quality problems in drinking water of China.

关键词： flavor profile analysis     2-methylisoborneol     swampy/septic odor     earthy/musty odor     drinking water quality    

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A red water occurrence in drinking water distribution systems caused by changes in water source in Beijing

ZHANG Xiaojian,MI Zilong,WANG Yang,LIU Shuming,NIU Zhangbin,LU Pinpin,WANG Jun,GU Junnong,CHEN Chao

《环境科学与工程前沿（英文）》 2014年 第8卷 第3期   页码 417-426 doi: 10.1007/s11783-013-0558-4

摘要： A red water phenomenon occurred in several communities few days after the change of water source in Beijing, China in 2008. In this study, the origin of this problem, the mechanism of iron release and various control measures were investigated. The results indicated that a significant increase in sulphate concentration as a result of the new water source was the cause of the red water phenomenon. The mechanism of iron release was found that the high-concentration sulphate in the new water source disrupted the stable shell of scale on the inner pipe and led to the release of iron compounds. Experiments showed that the iron release rate in the new source water within pipe section was over 11-fold higher than that occurring within the local source water. The recovery of tap water quality lasted several months despite ameliorative measures being implemented, including adding phosphate, reducing the overall proportion of the new water source, elevating the pH and alkalinity, and utilizing free chlorine as a disinfectant instead of chloramine. Adding phosphate was more effective and more practical than the other measures. The iron release rate was decreased after the addition of 1.5 mg·L orthophosphate- P, tripolyphosphate-P and hexametaphosphate-P by 68%, 83% and 87%, respectively. Elevating the pH and alkalinity also reduced the iron release rate by 50%. However, the iron release rate did not decreased after replacing chloramine by 0.5–0.8 mg·L of free chlorine as disinfectant.

关键词： iron release     drinking water distribution system     sulphate     phosphate     red water control     water quality stability    

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Nanofiltration for drinking water treatment: a review

《化学科学与工程前沿（英文）》 2022年 第16卷 第5期   页码 681-698 doi: 10.1007/s11705-021-2103-5

摘要： In recent decades, nanofiltration (NF) is considered as a promising separation technique to produce drinking water from different types of water source. In this paper, we comprehensively reviewed the progress of NF-based drinking water treatment, through summarizing the development of materials/fabrication and applications of NF membranes in various scenarios including surface water treatment, groundwater treatment, water reuse, brackish water treatment, and point of use applications. We not only summarized the removal of target major pollutants (e.g., hardness, pathogen, and natural organic matter), but also paid attention to the removal of micropollutants of major concern (e.g., disinfection byproducts, per- and polyfluoroalkyl substances, and arsenic). We highlighted that, for different applications, fit-for-purpose design is needed to improve the separation capability for target compounds of NF membranes in addition to their removal of salts. Outlook and perspectives on membrane fouling control, chlorine resistance, integrity, and selectivity are also discussed to provide potential insights for future development of high-efficiency NF membranes for stable and reliable drinking water treatment.

关键词： nanofiltration     drinking water     disinfection byproducts     micropollutants     selectivity    

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Emergency drinking water treatment in source water pollution incident-technology and practice in China

Xiaojian ZHANG , Chao CHEN ,

《环境科学与工程前沿（英文）》 2009年 第3卷 第3期   页码 364-368 doi: 10.1007/s11783-009-0027-2

摘要： An investigation into emergency potable water treatment technologies was conducted to investigate China’s water pollution situation. In order to confirm optimum parameters, the technological efficiency of each pollutant was obtained. About 100 contaminants were tested to find the emergency treatment technologies, most of which were found to be positive. This paper presents the three largest and most significant water pollution incidents in China to date, analyzing cases such as the nitrobenzene pollution incident in the Songhua River in November 2005, the cadmium pollution incident in the Beijiang River in December 2005, and the water crisis with odorous tap water in Wuxi City in May 2007.

关键词： emergency drinking water treatment     water pollution     adsorption     oxidation     precipitation    

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What have we known so far about microplastics in drinking water treatment? A timely review

《环境科学与工程前沿（英文）》 2022年 第16卷 第5期 doi: 10.1007/s11783-021-1492-5

摘要：

• 23 available research articles on MPs in drinking water treatment are reviewed.

关键词： Microplastics     Drinking water treatment     Coagulation     Flocculation     Membrane     Filtration    

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Potential shift of bacterial community structure and corrosion-related bacteria in drinking water distributionpipeline driven by water source switching

Yue Hu, Ding Dong, Kun Wan, Chao Chen, Xin Yu, Huirong Lin

《环境科学与工程前沿（英文）》 2021年 第15卷 第2期 doi: 10.1007/s11783-020-1320-3

摘要： Abstract • Bacterial release from aged pipe sections under extreme conditions was quantified. • Released bacterial community structure exhibited large variation after transition. • Risks from transition reduced significantly with cleaner source. As a result of pollution in the present water sources, cities have been forced to utilize cleaner water sources. There are few reports regarding the potential shift of bacterial community structure driven by water source switching, especially that of corrosion-related bacteria. Three types of finished water were used for simulation, the polluted source water from the Qiantang and Dongtiaoxi Rivers (China) was replaced by cleaner water from Qiandao Lake (China). Here, we discussed the transition effects through three simulated reactors. The bacterial characteristics were identified using the high-throughput sequencing and heterotrophic plate count method. It was observed that the level of culturable bacteria declined by 2–3 orders of magnitude after water source switching. The bacterial community released from the pipeline reactor was significantly different under different finished water, and it exhibited large variation at the genus level. Porphyrobacter (58.2%) and Phreatobacter (14.5%) clearly replaced Novosphingobium, Aquabacterium, and Cupriavidus as new dominant genera in system A, which could be attributed to the lower carbon and nitrogen content of the new water source. Although corrosion-inhibiting bacteria decreased after switching, they still maintained dominant in three reactors (6.6%, 15.9%, and 19.7%). Furthermore, potential opportunistic pathogens such as Sphingomonas were detected. Our study shows that after transition to a high quality water source, the total culturable bacteria released was in a downtrend, which leads to a great reduction in the risk of bacterial leakage in the produced drinking water.

关键词： Drinking water biosafety     Water source switching     Drinking water distribution system     Transition effects     High-throughput sequencing    

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Comparative genotoxicity of water processed by three drinking water treatment plants with different water

Ting Zhang, Heze Liu, Yiyuan Zhang, Wenjun Sun, Xiuwei Ao

《环境科学与工程前沿（英文）》 2020年 第14卷 第3期 doi: 10.1007/s11783-020-1214-4

摘要： Genotoxicity of substances is unknown in the water after treatment processes. Genotoxicity decreased by activated carbon treatment but increased by chlorination. Halogenated hydrocarbons and aromatic compounds contribute to genotoxicity. Genotoxicity was assessed by umu test; acute and chronic toxicity by ECOSAR. Inconsistent results confirmed that genotoxicity cannot be assessed by ECOSAR. Advanced water treatment is commonly used to remove micropollutants such as pesticides, endocrine disrupting chemicals, and disinfection byproducts in modern drinking water treatment plants. However, little attention has been paid to the changes in the genotoxicity of substances remaining in the water following the different water treatment processes. In this study, samples were collected from three drinking water treatment plants with different treatment processes. The treated water from each process was analyzed and compared for genotoxicity and the formation of organic compounds. The genotoxicity was evaluated by an umu test, and the acute and chronic toxicity was analyzed through Ecological Structure- Activity Relationship (ECOSAR). The results of the umu test indicated that biological activated carbon reduced the genotoxicity by 38%, 77%, and 46% in the three drinking water treatment plants, respectively, while chlorination increased the genotoxicity. Gas chromatograph-mass spectrometry analysis revealed that halogenated hydrocarbons and aromatic compounds were major contributors to genotoxicity. The results of ECOSAR were not consistent with those of the umu test. Therefore, we conclude that genotoxicity cannot be determined using ECOSAR .

关键词： Drinking water     Treatment process     Genotoxicity     Umu test     Ecological Structure-Activity Relationship    

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dissemination and removal of antibiotic resistant bacteria and antibiotic resistance genes in urban drinkingwater system: A review

Qiaowen Tan, Weiying Li, Junpeng Zhang, Wei Zhou, Jiping Chen, Yue Li, Jie Ma

《环境科学与工程前沿（英文）》 2019年 第13卷 第3期 doi: 10.1007/s11783-019-1120-9

摘要：

Reviewed the change of ARGs and ARB in full-scale urban drinking water systems.

Conventional processes are more promising than BAC process in ARGs removal.

Mechanisms of ARGs enrichment and spread in BAC filter and DWDSs are discussed.

Raise the need of future research on ARGs and ARB change in building plumbing systems.

关键词： Antibiotic resistant bacteria     Antibiotic resistance genes     Water source     Drinking water treatment plant     Drinking water distribution system     Urban drinking water system    

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Seasonal and treatment-process variations in invertebrates in drinking water treatment plants

Zhiling Wu, Xianchun Tang, Hongbin Chen

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1354-6

摘要： Abstract • Seasonal and treatment-process variations in invertebrates in a DWTP were analyzed. • The propagation and leakage of invertebrates in BAC filter were the most serious. • Invertebrates can survive and reproduce in chlorine disinfected clear water tanks. • Proportions of endogenous invertebrates increased along the treatment process. Problems associated with excessive propagation and leakage of invertebrates in drinking water have received increasing attention in recent years. We performed a monthly survey of invertebrate abundance and taxa in the effluent of each treatment stage in a drinking water treatment plant between May 2015 and April 2016 and analyzed seasonal and treatment-process variations in invertebrates. The results showed that invertebrate abundances in raw water, effluent of the biological activated carbon (BAC) filter, and finished water significantly correlated with water temperature, whereas no correlation was observed between water temperature and invertebrate abundance in the effluents of the sedimentation tank and sand filter. The dominant taxa in the effluent of each treatment stage were rotifers, nematodes, and crustaceans. The sedimentation tank could efficiently remove invertebrates with an annual average removal rate of 92%. The propagation and leakage of invertebrates occurred in the sand and BAC filters but more seriously in the latter. The average reproduction rate in the BAC filter was 268.8% with rotifers as the taxon that leaked the most. Invertebrate survival and reproduction were also observed in the chlorine-disinfected clean water reservoir with an average reproduction rate of 41.9%. Owing to differences in chlorine resistance, the reproduction ability of the dominant taxa was in the order nematodes>crustaceans>rotifers. The proportion of endogenous invertebrates gradually increased along the treatment process. The average proportion of endogenous invertebrates in the finished water was higher than 79.0%. Our findings suggested that waterworks should pay more attention to endogenous invertebrate growth.

关键词： Invertebrates     Drinking water     Seasonal variations     Treatment process    

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Molecular analysis of bacterial community in the tap water with different water ages of a drinking water

Feng Wang, Weiying Li, Yue Li, Junpeng Zhang, Jiping Chen, Wei Zhang, Xuan Wu

《环境科学与工程前沿（英文）》 2018年 第12卷 第3期 doi: 10.1007/s11783-018-1020-4

摘要： Bacterial community in the drinking water distribution system (DWDS) was regulated by multiple environmental factors, many of which varied as a function of water age. In this study, four water samples with different water ages, including finished water (FW, 0 d) and tap water (TW) [TW1 (1 d), TW2(2 d) and TW3(3 d)], were collected along with the mains of a practical DWDS, and the bacterial community was investigated by high-throughput sequencing technique. Results indicated that the residual chlorine declined with the increase of water age, accompanied by the increase of dissolved organic matter, total bacteria counts and bacterial diversity (Shannon). For bacterial community composition, although Proteobacteria phylum (84.12%-97.6%) and Alphaproteobacteria class (67.42%-93.09%) kept dominate, an evident regular was observed at the order level. In detail, the relative abundance of most of other residual orders increased with different degrees from the start to the end of the DWDS, while a downward trend was uniquely observed in terms of Rhizobiales, who was inferred to be chlorine-resistant and be helpful for inhibiting pipes corrosion. Moreover, some OTUs were found to be closely related with species possessing pathogenicity and chlorine-resistant ability, so it was recommended that the use of agents other than chlorine or agents that can act synergically with chlorine should be developed for drinking water disinfection. This paper revealed bacterial community variations along the mains of the DWDS and the result was helpful for understanding bacterial ecology in the DWDS.

关键词： Bacterial community     Water age     High-throughput sequencing technique     Drinking water distribution system    

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Applying chemical sedimentation process in drinking water treatment plant to address the emergent arsenicspills in water sources

Pengfei LIN,Xiaojian ZHANG,Hongwei YANG,Yong LI,Chao CHEN

《环境科学与工程前沿（英文）》 2015年 第9卷 第1期   页码 50-57 doi: 10.1007/s11783-014-0733-2

摘要： Arsenic (As) spills occurred more frequently and sometimes polluted water sources in recent years in China. It is as urgent need to develop emergency treatment technologies to address the arsenic threat for large-scale water treatment plants. In response, we developed a chemical sedimentation technology to remove arsenic contaminants for water treatment plants. Bench-scale experiments were conducted to investigate the efficiency of arsenic removal and the influencing factors of the chemical sedimentation treatment process. The influencing factors included the choice and dosage of coagulants, the valence of arsenic and pH value of solution. The As(V) contaminants can be almost completely removed by ferric or alum coagulants. The As(III) contaminants are more recalcitrant to chemical sedimentation, 75% for ferric coagulant and 40% for alum coagulant. The quantitative results of arsenic removal load by different ferric or alum coagulants were presented to help determine the parameters for arsenic treatment technology. The dominant mechanism for arsenic removal is static combination, or adsorption of negative arsenic species onto positive ferric hydroxide or alum hydroxide flocs. The efficiency of this treatment technology has also been demonstrated by a real production test in one water treatment plant with arsenic-rich source water and one emergency response. This technology was verified to be quick to set-up, easy to operate and highly efficient even for high concentration of arsenic.

关键词： Arsenic spill     chemical sedimentation     coagulation     drinking water     emergency treatment    

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我国水生态环境安全保障对策研究

霍守亮, 张含笑, 金小伟, 曹晓峰, 吴丰昌

《中国工程科学》 2022年 第24卷 第5期   页码 1-7 doi: 10.15302/J-SSCAE-2022.05.001

摘要：

良好的水生态环境是实现中华民族永续发展的内在要求，是生态文明和“美丽中国”建设的重要基础。当前，我国水生态环境形势依然严峻，富营养化、饮用水源地污染、地下水与近海海域污染、新污染物、生态用水短缺等水生态环境问题未得到根本解决。本文系统解析了我国水生态环境总体形势和面临的主要问题，提出了以流域水生态环境质量改善为核心，综合考虑水质改善、水生态保护和水环境风险防控的战略思路、基本原则和战略目标，提出了包括开展重点流域“山水林田湖草沙”协同治理和整体修复科技攻关与示范、开展京津冀协同发展区水环境水生态质量整体提升科技攻关与示范、开展新时期饮用水安全保障科技攻关与示范在内的3 项重大科技工程建议。为推动我国水生态环境安全保障的顺利实施，研究建议：全面系统修订《地表水环境质量标准》，强化其在水生态文明建设中的引领作用；科学评估我国湖泊氮磷营养物的时空差异，实施差异化营养物标准；科学评估我国水生态现状，深化推进水生态监测和评估；构建基于大数据融合的饮用水安全保障智慧化监管平台，保障饮用水安全。

关键词： 水生态环境；生态文明；质量改善；水生态安全；饮用水安全    

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Effects of humic acid on residual Al control in drinking water treatment plants with orthophosphate addition

Wendong WANG, Hua LI, Zhenzhen DING, Xiaochang WANG, Rui LIU

《环境科学与工程前沿（英文）》 2012年 第6卷 第4期   页码 470-476 doi: 10.1007/s11783-012-0422-y

摘要： This study aimed to investigate the effects of humic acid (HA) on residual Al control in drinking water facilities that used orthophosphate addition. The results showed that adding orthophosphate was an effective method for residual Al control for the raw water without HA. When orthophosphate was added at 1.0 min before the addition of poly aluminum chloride (PACl), the concentrations of soluble aluminum (Sol-Al) and total aluminum (Tot-Al) residue were 0.08 and 0.086 mg·L , respectively; both were reduced by 46% compared with the control experiment. The presence of HA would notably increase the residual Al concentration. For the raw water with 5 mg·L of HA, the concentrations of Sol-Al and Tot-Al increased from 0.136 and 0.174 mg·L to 0.172 and 0.272 mg·L , respectively. For water with a HA concentration above 5 mg·L , orthophosphate was ineffective in the control of residual Al, though there were still parts of orthophosphate were removed in coagulation. The amounts of Al removal were positively correlated with the solids freshly formed in coagulation. Similar to the raw water without HA, the best Al control was obtained with orthophosphate salt added at 1.0 min before PACl. HA concentrations in the raw water, solution pH, and the orthophosphate dosage suitable for residual Al control by orthophosphate precipitation were also investigated.

关键词： coagulation     drinking water     humic acid     orthophosphate     residual Al    

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标题 作者 时间 类型 操作

Development and application of innovative technologies for drinking water quality assurance in China

QU Jiuhui, YIN Chengqing, YANG Min, LIU Huijuan

期刊论文

Effects of water quality on the coagulation performances of humic acids irradiated with UV light

Wendong WANG,Qinghai FAN,Zixia QIAO,Qin YANG,Yabo WANG,Xiaochang WANG

期刊论文

Occurrence of odor problems in drinking water of major cities across China

SUN Daolin,YU Jianwei,YANG Min,AN Wei,ZHAO Yunyun,LU Ning,YUAN Shengguang,ZHANG Dongqing

期刊论文

A red water occurrence in drinking water distribution systems caused by changes in water source in Beijing

ZHANG Xiaojian,MI Zilong,WANG Yang,LIU Shuming,NIU Zhangbin,LU Pinpin,WANG Jun,GU Junnong,CHEN Chao

期刊论文

Nanofiltration for drinking water treatment: a review

期刊论文

Emergency drinking water treatment in source water pollution incident-technology and practice in China

Xiaojian ZHANG , Chao CHEN ,

期刊论文

What have we known so far about microplastics in drinking water treatment? A timely review

期刊论文

Potential shift of bacterial community structure and corrosion-related bacteria in drinking water distributionpipeline driven by water source switching

Yue Hu, Ding Dong, Kun Wan, Chao Chen, Xin Yu, Huirong Lin

期刊论文

Comparative genotoxicity of water processed by three drinking water treatment plants with different water

Ting Zhang, Heze Liu, Yiyuan Zhang, Wenjun Sun, Xiuwei Ao

期刊论文

dissemination and removal of antibiotic resistant bacteria and antibiotic resistance genes in urban drinkingwater system: A review

Qiaowen Tan, Weiying Li, Junpeng Zhang, Wei Zhou, Jiping Chen, Yue Li, Jie Ma

期刊论文

Seasonal and treatment-process variations in invertebrates in drinking water treatment plants

Zhiling Wu, Xianchun Tang, Hongbin Chen

期刊论文

Molecular analysis of bacterial community in the tap water with different water ages of a drinking water

Feng Wang, Weiying Li, Yue Li, Junpeng Zhang, Jiping Chen, Wei Zhang, Xuan Wu

期刊论文

Applying chemical sedimentation process in drinking water treatment plant to address the emergent arsenicspills in water sources

Pengfei LIN,Xiaojian ZHANG,Hongwei YANG,Yong LI,Chao CHEN

期刊论文

我国水生态环境安全保障对策研究

霍守亮, 张含笑, 金小伟, 曹晓峰, 吴丰昌

期刊论文

Effects of humic acid on residual Al control in drinking water treatment plants with orthophosphate addition

Wendong WANG, Hua LI, Zhenzhen DING, Xiaochang WANG, Rui LIU

期刊论文